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Article Dans Une Revue Atmospheric Measurement Techniques Année : 2017

Comparison of different Aethalometer correction schemes and a reference multi-wavelength absorption technique for ambient aerosol data

Jorge Saturno
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Christopher Pöhlker
Samara Carbone
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Yafang Cheng
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Xuguang Chi
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Florian Ditas
Isabella Hrabě de Angelis
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Daniel Morán-Zuloaga
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Mira L Pöhlker
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Luciana V Rizzo
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David Walter
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Qiaoqiao Wang
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Paulo Artaxo
Paolo Prati
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Meinrat O Andreae

Résumé

Deriving absorption coefficients from Aethalome-ter attenuation data requires different corrections to compensate for artifacts related to filter-loading effects, scattering by filter fibers, and scattering by aerosol particles. In this study, two different correction schemes were applied to seven-wavelength Aethalometer data, using multi-angle absorption photometer (MAAP) data as a reference absorption measurement at 637 nm. The compensation algorithms were compared to five-wavelength offline absorption measurements obtained with a multi-wavelength absorbance an-alyzer (MWAA), which serves as a multiple-wavelength reference measurement. The online measurements took place in the Amazon rainforest, from the wet-to-dry transition season to the dry season (June–September 2014). The mean absorption coefficient (at 637 nm) during this period was 1.8 ± 2.1 Mm −1 , with a maximum of 15.9 Mm −1. Under these conditions, the filter-loading compensation was negligible. One of the correction schemes was found to artificially increase the short-wavelength absorption coefficients. It was found that accounting for the aerosol optical properties in the scattering compensation significantly affects the absorption Ångström exponent (å ABS) retrievals. Proper Aethalometer data compensation schemes are crucial to retrieve the correct å ABS , which is commonly implemented in brown carbon contribution calculations. Additionally, we found that the wavelength dependence of uncompensated Aethalome-ter attenuation data significantly correlates with the å ABS retrieved from offline MWAA measurements.
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Dates et versions

hal-01836081 , version 1 (12-07-2018)

Identifiants

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Jorge Saturno, Christopher Pöhlker, Dario Massabó, Joel Brito, Samara Carbone, et al.. Comparison of different Aethalometer correction schemes and a reference multi-wavelength absorption technique for ambient aerosol data. Atmospheric Measurement Techniques, 2017, 10 (8), pp.2837 - 2850. ⟨10.5194/amt-10-2837-2017⟩. ⟨hal-01836081⟩
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