Skip to Main content Skip to Navigation

Comparison of different Aethalometer correction schemes and a reference multi-wavelength absorption technique for ambient aerosol data

Abstract : Deriving absorption coefficients from Aethalome-ter attenuation data requires different corrections to compensate for artifacts related to filter-loading effects, scattering by filter fibers, and scattering by aerosol particles. In this study, two different correction schemes were applied to seven-wavelength Aethalometer data, using multi-angle absorption photometer (MAAP) data as a reference absorption measurement at 637 nm. The compensation algorithms were compared to five-wavelength offline absorption measurements obtained with a multi-wavelength absorbance an-alyzer (MWAA), which serves as a multiple-wavelength reference measurement. The online measurements took place in the Amazon rainforest, from the wet-to-dry transition season to the dry season (June–September 2014). The mean absorption coefficient (at 637 nm) during this period was 1.8 ± 2.1 Mm −1 , with a maximum of 15.9 Mm −1. Under these conditions, the filter-loading compensation was negligible. One of the correction schemes was found to artificially increase the short-wavelength absorption coefficients. It was found that accounting for the aerosol optical properties in the scattering compensation significantly affects the absorption Ångström exponent (å ABS) retrievals. Proper Aethalometer data compensation schemes are crucial to retrieve the correct å ABS , which is commonly implemented in brown carbon contribution calculations. Additionally, we found that the wavelength dependence of uncompensated Aethalome-ter attenuation data significantly correlates with the å ABS retrieved from offline MWAA measurements.
Complete list of metadatas

Cited literature [53 references]  Display  Hide  Download

https://hal.uca.fr/hal-01836081
Contributor : Joel Ferreira de Brito <>
Submitted on : Thursday, July 12, 2018 - 9:02:45 AM
Last modification on : Wednesday, March 4, 2020 - 12:10:03 PM
Document(s) archivé(s) le : Monday, October 15, 2018 - 2:36:36 PM

File

2017_Saturno.pdf
Publisher files allowed on an open archive

Identifiers

Collections

Citation

Jorge Saturno, Christopher Pöhlker, Dario Massabó, Joel Brito, Samara Carbone, et al.. Comparison of different Aethalometer correction schemes and a reference multi-wavelength absorption technique for ambient aerosol data. Atmospheric Measurement Techniques, European Geosciences Union, 2017, 10 (8), pp.2837 - 2850. ⟨10.5194/amt-10-2837-2017⟩. ⟨hal-01836081⟩

Share

Metrics

Record views

307

Files downloads

276